Published graphical abstract comparing fracture in monolayer amorphous carbon nanocomposites with other two-dimensional materials.
Graphical abstract from Shin et al., Matter 8, 102000 (2025). Bo Ni, Bongki Shin, and Chee-Tat Toh contributed equally. Full authorship appears in the paper.

The central idea

Monolayer amorphous carbon is an in-plane nanocomposite: crystalline regions sit within an amorphous matrix. Their arrangement changes how a crack advances. Local blunting, deflection, and bridging create routes for energy absorption within the sheet itself.

What the work shows

In situ SEM tensile experiments report stable crack propagation and an energy release rate about eight times the graphene comparison used in the study. Molecular dynamics identifies crack-scale mechanisms and shows how the relative areas and sizes of crystalline and amorphous domains change fracture resistance.

Uniaxial tensile simulation of a MAC sheet without a pre-crack. Supplied Video S4, corresponding to the unnotched simulation discussed with Figure S7 in the paper. Original colors and forward frame sequence.

My contribution

I contributed equally to this collaborative study and conducted the molecular dynamics simulations with Zhenze Yang, under Markus J. Buehler, as stated in the published author-contribution record.

Scope of the result

The experimental fracture-energy comparison and the molecular simulation estimates refer to different sample scales and conditions. The simulations support the mechanisms and structural trends; they are not a numerical reproduction of every experimental value.